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Using the ab initio MO-LCAO-SCF-CISD method with a 6-31G** basis set we calculated, for 30 different N...N distances, the NH potentials of an [H2NH...NH2]- model complex containing a linear NH...N H-bond. Based on these potentials we quantized the NH stretching vibration by the...
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Thermolysis of Ru(IEt2Me2)(PPh3)2(CO)H2 (IEt2Me2 = 1,3-bis(ethyl)-4,5-dimethylimidazol-2-ylidene) in the presence of CH2CHSiMe3 results in C−H activation of an NCH2CH2−H bond; the process can be reversed by H2 or alcohols to give different isomers of the starting dihydride...
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