Here, we report a faceted Mo-doped BiVO4(Mo:BiVO4) with dual cocatalysts selectively loaded on its reduction and oxidation facets (Fig.1a). BiVO4is a photocatalyst with a suitable band structure and relatively narrow band-gap (2.4 eV) for H2O2photosynthesis, yet the reported efficiency rema...
The photosynthesis of hydrogen peroxide (H_2O_2) through the selective 2e~- oxygen reduction reaction (ORR) from O_2 and H_2O stands out as an environmentally sustainable and cost-effective method for generating this essential chemical.Unfortunately,the widespread application of most photocatalysts...
This work was primarily supported by the Artificial Photosynthesis Project of the New Energy and Industrial Technology Development Organization (NEDO) and also received funding from a Grant-in-Aid for Scientific Research (A) (No. 16H02417) and a Grant-in-Aid for Scientific Research (C) (No....
Tailoring Grain Boundary Chemistry of Polymeric Carbon Nitride for Enhanced Solar H2 Production and CO2 Reduction Angew. Chem. Int. Ed, 58 (2019), pp. 3433-3437 Google Scholar [8] Y. Li, T. Kong, S. Shen Artificial Photosynthesis with Polymeric Carbon Nitride: When Meeting Metal Nanoparticles...
Our work thus provides a promising avenue toward sustainable and high-efficiency artificial photosynthesis, contributing to the broader goal of sustainable energy solutions. 展开 关键词: PARTICULATE PHOTOCATALYST SHEETS ENERGY-CONVERSION ELECTRON MEDIATOR PHOTOANODE SRTIO3 BIVO4 年份: 2024 ...
Water splitting–biosynthetic system with CO2 reduction efficiencies exceeding photosynthesis Science, 352 (2016), pp. 1210-1213 CrossrefView in ScopusGoogle Scholar 2 K.K. Sakimoto, A.B. Wong, P. Yang Self-photosensitization of nonphotosynthetic bacteria for solar-to-chemical production Science, 35...
Converting solar energy into hydrogen (H2) by photocatalytic water splitting is a promising approach to simultaneously address the increasing energy demand
the oxygen reduction reaction(ORR)and water oxidation reaction(WOR),greatly restricts the efficiency of photocatalytic H2O2 production.In this highlight,we discuss the significant ad-vances in molecular engineering of carbon nitrides for H2O2 photosynthesis and the importance of the deep understan...
Metal–organic frameworks (MOFs) have been studied extensively in the hydrogen evolution reaction (HER) and the water oxidation reaction (WOR) with sacrificial reagents, but overall photocatalytic water splitting using MOFs has remained challenging, principally because of the fast recombination of photo-...
Guo3 & Z. Mi1 Solar water splitting is one of the key steps in artificial photosynthesis for future carbon- neutral, storable and sustainable source of energy. Here we show that one of the major obstacles for achieving efficient and stable overall water splitting over the emerging nanostructured...