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Figure 1. O–O bond formation in Co4O4 cubane (A) Structure of the [Co4O4Py4Ac4]0 (1) water oxidation catalyst. (B) O–O bond formation via the geminal hydroxide on the Co center. (C) O–O bond formation via radical coupling at adjacent Co centers in the high oxidation state....
Alternatively, the 2e(-) reductive cleavage of the O-O bond has a much larger driving force which minimizes this barrier and accelerates the rate of this reaction by approximately 10(7) in the native enzyme. This large difference in rate for the 2e(-) versus 1e(-) process supports a ...
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近日,来自西安交通大学的戴正飞研究员和西北工业大学的瞿永泉教授合作,在国际知名期刊ACS Nano上发表题为“Enlarging the Ni−O Bond Polarizability in a Phosphorene-Hosted Metal−Organic Framework for Boosted Water Oxidation Electrocatalysis”的文章。该工作通过基于清晰的物理化学图像和理论计算设计了镍基-MOFs/...
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Zhang-Long Yu, Yong-Feng Cheng, Ji-Ren Liu, Wu Yang, Dan-Tong Xu, Yu Tian, Jun-Qian Bian, Zhong-Liang Li, Li-Wen Fan, Cheng Luan, Ang Gao, Qiang-Shuai Gu,* Xin-Yuan Liu*. Cu(I)-Catalyzed Chemo- and Enantioselective Desymmetrizing C−O Bond Coupling of Acyl Radicals.J. Am...