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oxide growth is dictated by the reprecipitation process and therefore linked to the dissolution rate. Dissolution kinetics. in turn, tracks with the thermodynamic driving force, which increases with voltage and acidity.
For simplicity, the cation dissolution barriers under zero driving force were set to match the hopping barriers within the oxide. To compute accurate reference energy levels at the alloy-oxide boundary, we first used the recipe of ref. 71 to apply an energy shift of 1.36 eV to the O2 ...
(Ni3C) coated with a graphitic shell and deposited on a carbon platform. Our findings underscore the prominent role of nickel species, including Ni0, Ni2+, and Ni3+, in driving the catalytic activity. Notably, the catalyst exhibits an overpotential of 170 mV, a Tafel slope of 49 mV·...
Nickel-catalyzed C–H bond functionalization reactions provide an impressive alternative to those with noble metal catalysts due to their unique reactivity and low cost. However, the regioselective C(sp2)–H borylation reaction of arenes accomplished by
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In contrast, the anionic species becomes present in high percent within the pH range of 3–7, suggesting that the inner-sphere surface complexation is the main reason as a driving force for Ni2+ or Cd2+ uptake by iron oxide85. The effect of pH on the removal percentage of Cd2+ and Ni...
increased leading to faster saturation of the binding sites78. In other words, increase in influent metal concentration obviously enhanced the removal rate of the metal ions due to the corresponding increase in the driving force for mass transfer79. Remarkably, Table7reveals that the optimal column...