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dissociation being faster than energy redistribution, forming fragments with high kinetic energy but low internal energy.;The picosecond dynamics of energy redistribution in 1,4-dichlorobenzene and other polyatomics is examined by a two-color optical delay multiphoton absorption mass spectrometry experiment...
The results suggest a relatively simple dynamical picture for exothermic atom + polyatomic scattering, i.e., that of early barrier dynamics in atom + diatom systems but modified by impulsive recoil coupling at the transition state between translational/rotational degrees of freedom....
1) Intense laser-matter interactions for polyatomic molecules in the gas phase in order to determine to what extent processes like excitation, ionization and fragmentation can be controlled by modifying the phase and amplitude of the laser field according to the timescales for electronic, vibrational ...