该研究深入理解了酸性CO2RR中催化剂表面微环境的影响机制，并为设计酸性电解质中的稳定催化剂提供了指导。相关研究成果以“酸性CO2还原反应中动态催化剂微环境变化观察”（Observation on microenvironment changes of dynamic catalysts in acidic CO2 reduction）为题，发表于《美国化学会志》（Journal of the American Ch...
本研究提供了对CO2电解槽中水和离子传输动态的见解，并提出了不同的材料优化策略，为未来的实验提供了信息。文献信息 标题：Exploring CO2 reduction and crossover in membrane electrode assemblies 期刊：Nature Chemical Engineering DOI：10.1038/s44286-024-00062-0 ...
近日,课题组在Applied Catalysis B: Environment and Energy上发表了题为“Fine-tuning copper dispersion in Cu/SiO2core-shell particles regulates electrochemical CO2reduction product selectivity”的研究论文。文章的第一作者为2021级硕士...
In this Review, we analyse the state of the art in the implementation of low-dimensional nanomaterials and their van der Waals heterostructures for hydrogen evolution and CO2 reduction by electrocatalysis and photocatalysis. We explore the mechanisms involved in both reactions and the different ...
文献信息 Shoufu Cao et.al Precise electronic structure modulation on MXene-based single atom catalysts for high-performance electrocatalytic CO2 reduction reaction: A first-principle study Journal of Colloid and Interface Science 2023
Bin Liu, Zhiming Wei, Jie Ding, Ziyi Wang, Anyang Wang, Li Zhang, Yuhang Liu, Yuzheng Guo, Xuan Yang, Yueming Zhai,Enhanced Electrochemical CO2Reduction to Formate over Phosphate‐Modified In: Water Activation and Active Site Tuning, Angew. ...
Electrifying Model Single-Atom Catalyst for Elucidating the CO2Reduction Reaction Song Liu, Hongbin Yang, Sung-Fu Hung, Jie Ding, Weizheng Cai, Linghui Liu, Jiajian Gao, Xuning Li, Xinyi Ren, Zhichong Kuang, Yanqiang Huang, Tao Zhang, Bin Liu ...
图12 ATR transmission spectra in saturated CO2 0.1 M KCl electrolyte at different potentials showing the peaks that belong to the CO2 reduction intermediates. The background for these spectra was taken after 30 min at the same potential under a nitrogen purge[14] ...
2. Liu, C., Colón, B. C., Ziesack, M., Silver, P. A. and Nocera, D. G. (2016). Water splitting–biosynthetic system with CO2 reduction efficiencies exceeding photosynthesis. Science 352, 1210-1213. 3. White, J. L., Baruch, M. F., Pander III, J. E., Hu, Y., Fortmeyer...
电催化作为一种有效的人工固定CO2方式备受瞩目。但是,电催化CO2还原(Electrochemical CO2reduction, CO2RR)涉及复杂的多步质子耦合电子转移步骤,还原产物众多(气相产物,如CO、CH4;液相产物,如甲酸和醇类等)。甲醇作为CO2RR过程最有价值的C1产物,其能量密度高,易于常压储存,并可直接用于燃料电池。但是电催化CO2至甲醇...