Electronic configuration is crucial for enhancing the catalytic activities of spinels for the oxygen evolution reaction (OER). However, controlling the electronic spin state of materials is still a challenge. In this work, we synthesized Fe-doped meso-Co3O4via a nanocasting method. The merit of ...
et al. Impact of the 3d electronic states of cobalt and manganese phthalocyanines on the electronic structure at the interface to Ag(111). J. Phys. Chem. C 115, 21334–21340 (2011). Article CAS Google Scholar Petraki, F. et al. Modification of the 3d-electronic configuration of ...
4f electronic configurationBaCeO3CocatalystThe perovskite-type photocatalyst BaCeO3, prepared by a Pechini method, was investigated for CO2 reduction under UV light irradiation. The prepared samples were characterized by X-ray diffraction, BET surface area measurement, UV–vis reflectance spectroscopy, ...
The CO2 electroreduction reaction (CO2RR) to fuels and feedstocks is an attractive route to close the anthropogenic carbon cycle and store renewable energy. The generation of more reduced chemicals, especially multicarbon oxygenate and hydrocarbon produc
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The potential energy function of the 1 Σ excited state of CO , which lies around 11 eV above the electronic ground state, has been investigated by ab initio multiconfiguration self-consistent field calculations. It has been found that this state exhibits two minima on one-dimensional cuts of ...
On this configuration, as shown in Figure 5F, the CO2 adsorption energy was maximized at −0.46 eV, which is significantly stronger than on sites with adjacent Cu-Cu atoms (−0.31 eV).82 Additionally, the Pd atoms had a significant electronic effect on the isolated Cu, causing an ...
SACs normally exhibit higher catalytic performances because of the high ratio of low-coordinated configurations8,45,46. However, the transition metals have to be screened since only the SACs with well balanced empty/occupieddorbitals can exhibit optimal catalytic performance. To find suitable SACs, 29...
Advanced catalyst design and reactor configuration upgrade in electrochemical carbon dioxide conversion. Adv. Mater. https://doi.org/10.1002/adma.202303052 (2023). Endrodi, B. et al. Operando cathode activation with alkali metal cations for high current density operation of water-fed zero-gap ...